Low Field Magnetic Response of the Granular Superconductor LaSrCuO

The properties of the low excitation field magnetic response of the granular high temperature (HTSC) superconductor LaSrCuO have been analyzed at low temperatures. The response of the Josephson currents has been extracted from the data. It is shown that intergrain current response is fully irreversible, producing shielding response, but do not carry Meissner magnetization. Analysis of the data shows that the system of Josephson currents freezes into a glassy state even in the absense of external magnetic field, which is argued to be a consequence of the d-wave nature of superconductivity in LaSrCuO. The macroscopic diamagnetic response to very weak variations of the magnetic field is shown to be strongly irreversible but still qualitatively different from any previously known kind of the critical-state behaviour in superconductors. A phenomenological description of these data is given in terms of a newly proposed ``fractal'' model of irreversibility in superconductors.Comment: LATEX, twocolumns, 22 pages including 20 eps-figure

Second harmonics and compensation effect in ceramic superconductors

A three-dimensional lattice of the Josephson junctions with a finite self-conductance is employed to model the ceramic superconductors. The nonlinear ac susceptibility and the compensation effect are studied by Monte Carlo simulations in this model. The compensation effect is shown to be due to the existence of the chiral glass phase. We demonstrate, in agreement with experiments, that this effect may be present in the ceramic superconductors which show the paramagnetic Meissner effect.Comment: 6 pages, latex, 4 figures, Phys. Rev. B (accepted

Electric field dependence of thermal conductivity of a granular superconductor: Giant field-induced effects predicted

The temperature and electric field dependence of electronic contribution to the thermal conductivity (TC) of a granular superconductor is considered within a 3D model of inductive Josephson junction arrays. In addition to a low-temperature maximum of zero-field TC K(T,0) (controlled by mutual inductance L_0 and normal state resistivity R_n), the model predicts two major effects in applied electric field: (i) decrease of the linear TC, and (ii) giant enhancement of the nonlinear (i.e., grad T-dependent) TC with [K(T,E)-K(T,0)]/K(T,0) reaching 500% for parallel electric fields E=E_T (E_T=S_0|grad T| is an "intrinsic" thermoelectric field). A possiblity of experimental observation of the predicted effects in granular superconductors is discussed.Comment: 5 LaTeX pages (jetpl.sty included), 2 EPS figures. To be published in JETP Letter

Microwave dielectric study of spin-Peierls and charge ordering transitions in (TMTTF)2_2PF6_6 salts

We report a study of the 16.5 GHz dielectric function of hydrogenated and deuterated organic salts (TMTTF)$_2$PF$_6$. The temperature behavior of the dielectric function is consistent with short-range polar order whose relaxation time decreases rapidly below the charge ordering temperature. If this transition has more a relaxor character in the hydrogenated salt, charge ordering is strengthened in the deuterated one where the transition temperature has increased by more than thirty percent. Anomalies in the dielectric function are also observed in the spin-Peierls ground state revealing some intricate lattice effects in a temperature range where both phases coexist. The variation of the spin-Peierls ordering temperature under magnetic field appears to follow a mean-field prediction despite the presence of spin-Peierls fluctuations over a very wide temperature range in the charge ordered state of these salts.Comment: 7 pages, 6 figure

Nonlinear Seebeck Effect in a Model Granular Superconductor

The change of the Josephson supercurrent density of a weakly-connected granular superconductor in response to externally applied arbitrary thermal gradient dT/dx (nonlinear Seebeck effect) is considered within a model of 3D Josephson junction arrays. For dT/dx>(dT/dx)_c, where (dT/dx)_c is estimated to be of the order of 10^4 K/m for YBCO ceramics with an average grain's size of 10 microns, the weak-links-dominated thermopower S (Seebeck coefficient) is predicted to become strongly dT/dx-dependent.Comment: REVTEX, no figure

A new quantum fluid at high magnetic fields in the marginal charge-density-wave system α\alpha-(BEDT-TTF)2M_2MHg(SCN)4_4 (where M=M=~K and Rb)

Single crystals of the organic charge-transfer salts $\alpha$-(BEDT-TTF)$_2M$Hg(SCN)$_4$ have been studied using Hall-potential measurements ($M=$K) and magnetization experiments ($M$ = K, Rb). The data show that two types of screening currents occur within the high-field, low-temperature CDW$_x$ phases of these salts in response to time-dependent magnetic fields. The first, which gives rise to the induced Hall potential, is a free current (${\bf j}_{\rm free}$), present at the surface of the sample. The time constant for the decay of these currents is much longer than that expected from the sample resistivity. The second component of the current appears to be magnetic (${\bf j}_{\rm mag}$), in that it is a microscopic, quasi-orbital effect; it is evenly distributed within the bulk of the sample upon saturation. To explain these data, we propose a simple model invoking a new type of quantum fluid comprising a CDW coexisting with a two-dimensional Fermi-surface pocket which describes the two types of current. The model and data are able to account for the body of previous experimental data which had generated apparently contradictory interpretations in terms of the quantum Hall effect or superconductivity.Comment: 13 pages, 11 figure

Charge ordering, symmetry and electronic structure issues and Wigner crystal structure of the quarter-filled band Mott insulators and high pressure metals δ-(EDT-TTF-CONMe2)2X, X = Br and AsF6

We report on the synthesis and application of an internal chemical pressure to effectively control, and reduce, the Mott gap in the system δ-(EDT-TTF-CONMe2)2X, X = Br, AsF6; the detailed accounts of its Pmna, averaged room temperature structure and reversible phase transition at ca. 190 K towards a low tem

Ground state and finite temperature behavior of 1/4-filled band zigzag ladders

We consider the simplest example of lattice frustration in the 1/4-filled band, a one-dimensional chain with next-nearest neighbor interactions. For this zigzag ladder with electron-electron as well as electron-phonon interactions we present numerical results for ground state as well as thermodynamic properties. In this system the ground state bond distortion pattern is independent of electron-electron interaction strength. The spin gap in the ground state of the zigzag ladder increases with the degree of frustration. Unlike in one-dimension, where the spin-gap and charge ordering transitions can be distinct, we show that in the ladder they occur simultaneously. We discuss spin gap and charge ordering transitions in 1/4-filled materials with one, two, or three dimensional crystal structures. We show empirically that regardless of dimensionality the occurrence of simultaneous or distinct charge and magnetic transitions can be correlated with the ground state bond distortion pattern.Comment: 12 pages, 8 eps figure

Electromagnetic response of a conductor with complex conductivity

The aim of this paper is to describe the electromagnetic response of a conductor with complex conductivity. We will show how the geometry of the measuring apparatus can modify the amplitude of this response. We will particularly emphasize the role that plays a complex conductivity, as we can find in granular superconductors, on the mesured magnetic susceptibility of the sample.Cet article a pour but de décrire la réponse électromagnétique d'un conducteur muni d'une conductivité complexe. Nous montrerons comment la géométrie du dispositif de mesure peut modifier l'amplitude de cette réponse. Nous insisterons particulièrement sur le rôle que joue une conductivité complexe, comme nous pouvons en trouver dans les supraconducteurs granulaires, sur la susceptibilité magnétique mesurée de l'échantillon